Multi-harmonic near-infrared-ultraviolet dual-comb spectrometer

Kristina F. Chang, Daniel M. B. Lesko, Carter Mashburn, Peter Chang, Eugene Tsao, Alexander J. Lind, Scott A. Diddams

Abstract

Dual-comb spectroscopy in the ultraviolet (UV) and visible would enable broad bandwidth electronic spectroscopy with unprecedented frequency resolution. However, there are significant challenges in generation, detection, and processing of dual-comb data that have restricted its progress in this spectral region. In this work, we leverage robust 1550 nm few-cycle pulses to generate frequency combs in the UV–visible. We combine these combs with a wavelength multiplexed dual-comb spectrometer and simultaneously retrieve 100 MHz comb-mode-resolved spectra over three distinct harmonics at 386, 500, and 760 nm. The experiments highlight the path to continuous dual-comb coverage spanning 200–750 nm, offering extensive access to electronic transitions in atoms, molecules, and solids.